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The direct observation and interpretation of gas hydrate decomposition with ocean depth
Ma, L.1,2,3,4; Luan, Z.1,2,3,4; Du, Z.1,2,3; Zhang, X.1,2,3,4; Zhang, Y.1,2,3,4; Zhang, X.1,2,3,4
2023-08-25
发表期刊GEOCHEMICAL PERSPECTIVES LETTERS
ISSN2410-339X
卷号27页码:9-14
通讯作者Zhang, X.([email protected])
摘要An exposed gas hydrate (EGH) evolutional model as a function of water depth was established by in situ EGHs ascent experiments in cold seep areas of Haima (1509 m, 2.88 degrees C and 15.22 MPa), Lingshui (1760 m, 2.56 degrees C, 17.76 MPa and pH = 7.97) and Site F (1100 m, 3.57 degrees C, 11.09 MPa and pH = 7.69) in the South China Sea. A remotely operated vehicle was used to reproduce the in situ EGH ascent. Changes and temperature variations during EGH ascent were monitored in real time using a Raman insertion probe and dissolved oxygen sensor. The EGH ascent involved three stages of change: i) the metastable stage where no morphology changes, but where gas escapes and there is a decrease in internal temperature; ii) a second stage of coexistence of peripheral hydrate decomposition and internal hydrate growth; iii) a third stage of internal hydrate decomposition at shallower depths. Experimental results indicated that EGHs can carry gas bubbles to shallow depths and even to the sea surface. This could be an important transport mode for cold seep gases affecting shallow waters or the atmosphere.
DOI10.7185/geochemlet.2327
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[52001303]; National Natural Science Foundation of China[92058206]; National Natural Science Foundation of China[42221005]; National Natural Science Foundation of China[41822604]; National Natural Science Foundation of China[42049582]; Strategic Priority Research Program, CAS[XDB42040302]; Young Taishan Scholars Program[tsqn201909158]; Key Project of Ocean Research Center, Chinese Academy of Sciences[COMS2020J03]
WOS研究方向Geochemistry & Geophysics
WOS类目Geochemistry & Geophysics
WOS记录号WOS:001144160800002
出版者EUROPEAN ASSOC GEOCHEMISTRY
WOS关键词IN-SITU ; METHANE HYDRATE ; DEEP-SEA ; STABILITY ; BUBBLE ; CARBON ; SEEPS ; SLOPE ; VENT
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被引频次:3[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.qdio.ac.cn/handle/337002/184393
专题海洋地质与环境重点实验室
通讯作者Zhang, X.
作者单位1.Chinese Acad Sci, Inst Oceanol, Ctr Ocean Mega Sci, Key Lab Marine Geol & Environm, Qingdao 266071, Peoples R China
2.Chinese Acad Sci, Inst Oceanol, Ctr Deep Sea Res, Ctr Ocean Mega Sci, Qingdao 266071, Peoples R China
3.LaoShan Lab, Lab Marine Geol, Qingdao 266061, Peoples R China
4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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GB/T 7714
Ma, L.,Luan, Z.,Du, Z.,et al. The direct observation and interpretation of gas hydrate decomposition with ocean depth[J]. GEOCHEMICAL PERSPECTIVES LETTERS,2023,27:9-14.
APA Ma, L.,Luan, Z.,Du, Z.,Zhang, X.,Zhang, Y.,&Zhang, X..(2023).The direct observation and interpretation of gas hydrate decomposition with ocean depth.GEOCHEMICAL PERSPECTIVES LETTERS,27,9-14.
MLA Ma, L.,et al."The direct observation and interpretation of gas hydrate decomposition with ocean depth".GEOCHEMICAL PERSPECTIVES LETTERS 27(2023):9-14.
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