Building P-doped MoS2/g-C3N4 layered heterojunction with a dual-internal electric field for efficient photocatalytic sterilization

doi:10.1016/j.cej.2021.132588

	Building P-doped MoS2/g-C3N4 layered heterojunction with a dual-internal electric field for efficient photocatalytic sterilization
	Zhang, Xin 1; Tian, Fenyang 1; Lan, Xiao2 ; Liu, Yequn 3; Yang, Weiwei 1; Zhang, Jie2 ; Yu, Yongsheng 1
	2022-02-01
发表期刊	CHEMICAL ENGINEERING JOURNAL
ISSN	1385-8947
卷号	429 页码:7
通讯作者	Yang, Weiwei([email protected]) ; Zhang, Jie([email protected]) ; Yu, Yongsheng([email protected])
摘要	The construction of internal electric field (IEF) is usually considered an effective strategy to enhance photocatalytic efficiency because of its significant role in photo-induced carrier separation. Herein, we report a novel method to synthesize phosphorus-doped (P-doped) MoS2/g-C3N4 layer-by-layer composite, which could expose more active sites and generate a strong interaction by forming Mo-N bonds for photocatalytic sterilization. It is experimentally and theoretically confirmed that P-doped MoS2/g-C3N4 heterojunctions not only generate a dualIEF to drive charge migration, but also facilitate spatially separated redox sites to further promote the separation of photo-induced carrier. The optimized P-doped MoS2/g-C3N4 layered heterojunction exhibits high photocatalytic sterilization efficiency (99.99%) towards E. coli under visible-light irradiation, which is remarkably higher compared with those of P-doped g-C3N4 (44.73%) and P-doped MoS2 (61.69%), respectively. This research will offer a novel method of designing and synthesizing layered composite photocatalyst with a dual-IEF for effective photocatalytic sterilization.
关键词	Layered heterojunction Dual-internal electric field Separated redox sites Photocatalytic sterilization P-doped MoS2 g-C3N4
DOI	10.1016/j.cej.2021.132588
收录类别	SCI
语种	英语
资助项目	National Natural Science Foundation of China[51871078]; National Natural Science Foundation of China[52071119]; National Natural Science Foundation of China[42076043]; Heilongjiang Science Foundation[LH2020B006]
WOS研究方向	Engineering
WOS类目	Engineering, Environmental ; Engineering, Chemical
WOS记录号	WOS:000729803400001
出版者	ELSEVIER SCIENCE SA
引用统计	被引频次：167[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.qdio.ac.cn/handle/337002/177507
专题	海洋环境腐蚀与生物污损重点实验室
通讯作者	Yang, Weiwei; Zhang, Jie; Yu, Yongsheng
作者单位	1.Harbin Inst Technol, Sch Chem & Chem Engn, MIIT Key Lab Crit Mat Technol New Energy Convers, Harbin 150001, Heilongjiang, Peoples R China 2.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, Qingdao 266071, Shandong, Peoples R China 3.Chinese Acad Sci, Analyt Instrumentat Ctr, Inst Coal Chem, State Key Lab Coal Convers, Taiyuan 030001, Shanxi, Peoples R China
通讯作者单位	海洋环境腐蚀与生物污损重点实验室
推荐引用方式 GB/T 7714	Zhang, Xin,Tian, Fenyang,Lan, Xiao,et al. Building P-doped MoS2/g-C3N4 layered heterojunction with a dual-internal electric field for efficient photocatalytic sterilization[J]. CHEMICAL ENGINEERING JOURNAL,2022,429:7.
APA	Zhang, Xin.,Tian, Fenyang.,Lan, Xiao.,Liu, Yequn.,Yang, Weiwei.,...&Yu, Yongsheng.(2022).Building P-doped MoS2/g-C3N4 layered heterojunction with a dual-internal electric field for efficient photocatalytic sterilization.CHEMICAL ENGINEERING JOURNAL,429,7.
MLA	Zhang, Xin,et al."Building P-doped MoS2/g-C3N4 layered heterojunction with a dual-internal electric field for efficient photocatalytic sterilization".CHEMICAL ENGINEERING JOURNAL 429(2022):7.

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