Combination of metal-organic framework with Ag-based semiconductor enhanced photocatalytic antibacterial performance under visible-light
Liu, Ning1,2,3; Zhang, Jie2,3; Wang, Yanhua1; Zhu, Qingjun2,3; Wang, Chunli2,3; Zhang, Xuan1; Duan, Jizhou2,3; Hou, Baorong2,3; Sheng, Jinlu4
2022-07-05
发表期刊COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
ISSN0927-7757
卷号644页码:8
通讯作者Zhang, Jie([email protected]) ; Wang, Yanhua([email protected])
摘要In this study, visible-light-sensitive Ag/AgCl@ZIF-8 catalysts were prepared by one-pot reactions combined with photo-reduction processes. The photocatalysts were tested by XRD, SEM, HRTEM, UV-DRS, XPS. It can be observed that the 2-methylimidazole zinc salt(ZIF-8)exhibited the rhombic dodecahedron morphology with Ag/AgCl or AgCl nanoparticle evenly distributed around it. The composite photocatalyst Ag/AgCl@ZIF-8 sample showed excellent photocatalytic antibacterial performance. Under the condition of illumination for 90 min, the composite material can inactivate almost all P. aeruginosaudomonas aeruginosa (P.aeruginosa), Escherichia coli(E. coli) and Staphylococcus aureus (S. aureus). Moreover, the Ag/AgCl@ZIF-8 photocatalyst had excellent stability and reusability in the cyclic degradation experiment. The possible photocatalysis principle was given on the basic of ROS quenching experiment and electron paramagnetic resonance (EPR) tests, demonstrating that the.O-2(-)& nbsp;and h(+) were the main active substance. This result provides a new way for the development of MOF-based composites for antibacterial applications.
关键词Photocatalysis Metal-organic frameworks Ag-based semiconductors composite Photocatalytic antibacterial
DOI10.1016/j.colsurfa.2022.128813
收录类别SCI
语种英语
资助项目National Nat-ural Science Foundation of China[42076043]; Shandong Provincial Natural Science Foundation[ZR2020MD080]
WOS研究方向Chemistry
WOS类目Chemistry, Physical
WOS记录号WOS:000796609500006
出版者ELSEVIER
引用统计
被引频次:11[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.qdio.ac.cn/handle/337002/179288
专题海洋环境腐蚀与生物污损重点实验室
通讯作者Zhang, Jie; Wang, Yanhua
作者单位1.Ocean Univ China, Coll Chem & Chem Engn, Key Lab Marine Chem Theory & Technol, Minist Educ, Qingdao 266100, Peoples R China
2.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, Qingdao 266071, Peoples R China
3.Pilot Natl Lab Marine Sci & Technol Qingdao, Open Studio Marine Corros & Protect, 1 Wenhai Rd, Qingdao 266237, Peoples R China
4.Chongqing JiaoTong Univ, Sch Traff & Tansportat, Chongqing 400074, Peoples R China
第一作者单位中国科学院海洋研究所
通讯作者单位中国科学院海洋研究所
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GB/T 7714
Liu, Ning,Zhang, Jie,Wang, Yanhua,et al. Combination of metal-organic framework with Ag-based semiconductor enhanced photocatalytic antibacterial performance under visible-light[J]. COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS,2022,644:8.
APA Liu, Ning.,Zhang, Jie.,Wang, Yanhua.,Zhu, Qingjun.,Wang, Chunli.,...&Sheng, Jinlu.(2022).Combination of metal-organic framework with Ag-based semiconductor enhanced photocatalytic antibacterial performance under visible-light.COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS,644,8.
MLA Liu, Ning,et al."Combination of metal-organic framework with Ag-based semiconductor enhanced photocatalytic antibacterial performance under visible-light".COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS 644(2022):8.
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