Fabrication of an ultrathin 2D/2D C3N4/MoS2 heterojunction photocatalyst with enhanced photocatalytic performance

doi:10.1016/j.jallcom.2019.151681

	Fabrication of an ultrathin 2D/2D C3N4/MoS2 heterojunction photocatalyst with enhanced photocatalytic performance
	Li, Weibing 1,2; Wang, Lin1 ; Zhang, Qiang 1; Chen, Zhuoyuan 2,3,4; Deng, Xiaoyan 1; Feng, Chang2 ; Xu, Likun 2; Sun, Mingxian 2
	2019-11-05
发表期刊	JOURNAL OF ALLOYS AND COMPOUNDS
ISSN	0925-8388
卷号	808 页码:9
通讯作者	Feng, Chang([email protected])
摘要	An ultrathin 2D/2D C3N4/MoS2 (U-CN/MoS2) heterojunction photocatalyst was prepared by a simple mechanical grinding technique to investigate the photocatalytic degradation RhB and hydrogen production performance. Physical characterization shows that the ultrathin MoS2 nanosheets (U-MoS2) can form heterojunction with the ultrathin C3N4 (U-CN), and their intrinsic crystal structure remains stable. Further photocatalytic performance test demonstrated that the U-CN/MoS2 heterojunction photocatalyst significantly enhanced the photocatalytic activity of U-CN. The U-CN/MoS2 photocatalyst with 3% mass fraction of MoS2 station (U-CN/MoS2-3) has the optimal photocatalytic performance. Due to MoS2 has a suitable band structure and can replace noble metal as a co-catalyst, the U-CN/MoS2-3 could achieve the hydrogen production efficiency of 385.04 mu mol.h(-1).g(-1), which makes MoS2 show potential in photocatalytic hydrogen production. The enhanced photocatalytic performance was attributed to the significantly enhanced concentration of photogenerated carriers, the effective separation of photogenerated carriers, and suppressed recombination of photogenerated electrons and holes in the photocatalytic reaction. (C) 2019 Elsevier B.V. All rights reserved.
关键词	Heterojunction photocatalysts Ultrathin C3N4/MoS2 Mechanical grinding Photocatalytic performance
DOI	10.1016/j.jallcom.2019.151681
收录类别	SCI
语种	英语
资助项目	State Key Laboratory for Marine Corrosion and Protection, Luoyang Ship Material Research Institute, China[614290101011703]###28; State Key Laboratory for Marine Corrosion and Protection, Luoyang Ship Material Research Institute, China[KF160413]###29; State Key Laboratory for Marine Corrosion and Protection, Luoyang Ship Material Research Institute, China[KF160402]###30; National Natural Science Foundation of China[41576114]###32; National Natural Science Foundation of China[41376126]###31; Key Research and Development Program of Shandong Province[2018GSF117007]###3084; Qingdao Innovative Leading Talent Foundation[15-10-3-15-(39)-zch]###33; Qingdao Science and Technology Achievement Transformation Guidance Plan (Applied Basic Research)[14-2-4-4-jch]###34; State Key Laboratory for Marine Corrosion and Protection, Luoyang Ship Material Research Institute, China[614290101011703]; State Key Laboratory for Marine Corrosion and Protection, Luoyang Ship Material Research Institute, China[KF160413]; State Key Laboratory for Marine Corrosion and Protection, Luoyang Ship Material Research Institute, China[KF160402]; National Natural Science Foundation of China[41576114]; National Natural Science Foundation of China[41376126]; Key Research and Development Program of Shandong Province[2018GSF117007]; Qingdao Innovative Leading Talent Foundation[15-10-3-15-(39)-zch]; Qingdao Science and Technology Achievement Transformation Guidance Plan (Applied Basic Research)[14-2-4-4-jch]
WOS研究方向	Chemistry ; Materials Science ; Metallurgy & Metallurgical Engineering
WOS类目	Chemistry, Physical ; Materials Science, Multidisciplinary ; Metallurgy & Metallurgical Engineering
WOS记录号	WOS:000483694900032
出版者	ELSEVIER SCIENCE SA
引用统计	被引频次：55[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.qdio.ac.cn/handle/337002/162736
专题	海洋环境腐蚀与生物污损重点实验室
通讯作者	Feng, Chang
作者单位	1.Qingdao Univ Sci & Technol, Sch Environm & Safety Engn, 53 Zhengzhou Rd, Qingdao 266042, Shandong, Peoples R China 2.Luoyang Ship Mat Res Inst, State Key Lab Marine Corros & Protect, Wenhai Rd, Qingdao 266237, Shandong, Peoples R China 3.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, 7 Nanhai Rd, Qingdao 266071, Shandong, Peoples R China 4.Chinese Acad Sci, Ctr Ocean Mega Sci, 7 Nanhai Rd, Qingdao 266071, Shandong, Peoples R China
推荐引用方式 GB/T 7714	Li, Weibing,Wang, Lin,Zhang, Qiang,et al. Fabrication of an ultrathin 2D/2D C3N4/MoS2 heterojunction photocatalyst with enhanced photocatalytic performance[J]. JOURNAL OF ALLOYS AND COMPOUNDS,2019,808:9.
APA	Li, Weibing.,Wang, Lin.,Zhang, Qiang.,Chen, Zhuoyuan.,Deng, Xiaoyan.,...&Sun, Mingxian.(2019).Fabrication of an ultrathin 2D/2D C3N4/MoS2 heterojunction photocatalyst with enhanced photocatalytic performance.JOURNAL OF ALLOYS AND COMPOUNDS,808,9.
MLA	Li, Weibing,et al."Fabrication of an ultrathin 2D/2D C3N4/MoS2 heterojunction photocatalyst with enhanced photocatalytic performance".JOURNAL OF ALLOYS AND COMPOUNDS 808(2019):9.

条目包含的文件
文件名称/大小	文献类型	版本类型	开放类型	使用许可
Fabrication of an ul（2462KB）	期刊论文	出版稿	限制开放	CC BY-NC-SA	浏览
Fabrication of an ul（2462KB）	期刊论文	出版稿	限制开放	CC BY-NC-SA	浏览