Distribution, pollution status, and source apportionment of trace metals in lake sediments under the influence of the South-to-North Water Transfer Project, China

doi:10.1016/j.scitotenv.2019.03.306

	Distribution, pollution status, and source apportionment of trace metals in lake sediments under the influence of the South-to-North Water Transfer Project, China
	Zhuang, Wen 1,2,3; Ying, Samantha C.2; Frie, Alexander L.2; Wang, Qian3 ; Song, Jinming1 ; Liu, Yongxia 3; Chen, Qing 4; Lai, Xiaoying 5
	2019-06-25
发表期刊	SCIENCE OF THE TOTAL ENVIRONMENT
ISSN	0048-9697
卷号	671 页码:108-118
通讯作者	Zhuang, Wen([email protected])
摘要	In an effort to combat the threat of drought, China constructed the South-to-North Water Transfer Project (SNWTP), the biggest water transfer project in terms of volume with the largest beneficiary population in the world. Reports have shown that massive water diversion projects have had detrimental environmental consequences including water quality decline and freshwater habitat degradation. However, few reports have assessed the impact of the transfer project on sediment quality, which is highly susceptible to allogenic and local anthropogenic pollution. We examined the distribution characteristics of Cd, Cr, Cu, Ni, Pb and Zn in surface sediment of the largest reservoir along the East Route of SNWTP, Nansihu Lake, followed by positive matrix factorization (PMF) to determine their potential sources. We utilized enrichment factor, multiple sediment quality guidelines (SQGs), and potential ecological risk index (RI) to determine metal accumulation or pollution risk. The results show the mean concentrations of Cr, Cu, Pb, Zn were slightly lower than in samples collected in 2003, 2010 and 2012, while the mean concentrations of Cr and Ni were significantly higher than samples from previous years. Among the six metals, Cr, Cu and Ni are of higher ecological risk according to SQGs; but Cd is of higher ecological risk according to RI. PMF analysis shows that industrial production and shipping are important sources of Cr, Cu, and Ni. PMF analysis also shows that a considerable amount of trace metals, especially Cd, Cr, Pb and Zn, mainly comes from the use of pesticide fertilizers and biomass sources in farmland, and may partly enter Nansihu Lake from SNWTP. This study reveals the possible sources of trace metals to the Nansihu Lake which is part of SNWTP; the results of the study may serve as a reference for better understanding the impact of future water diversion projects on metals distribution. (C) 2019 Elsevier B.V. All rights reserved.
关键词	Trace metals Sediment pollution Source apportionment Water transfer project Nansihu Lake
DOI	10.1016/j.scitotenv.2019.03.306
收录类别	SCI
语种	英语
资助项目	Natural Science Foundation of Shandong Province, China[ZR2017QD012]###664; Natural Science Foundation of Shandong Province, China[ZR2014DP005]###665; Natural Science Foundation of Shandong Province, China[ZR2016CB29]###666; National Natural Science Foundation of China[31600080]###668; USDA NIFA Hatch Fund###1137; Natural Science Foundation of Shandong Province, China[ZR2017QD012]; Natural Science Foundation of Shandong Province, China[ZR2014DP005]; Natural Science Foundation of Shandong Province, China[ZR2016CB29]; National Natural Science Foundation of China[31600080]; USDA NIFA Hatch Fund
WOS研究方向	Environmental Sciences & Ecology
WOS类目	Environmental Sciences
WOS记录号	WOS:000466090500013
出版者	ELSEVIER SCIENCE BV
引用统计	被引频次：63[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.qdio.ac.cn/handle/337002/157034
专题	海洋生态与环境科学重点实验室
通讯作者	Zhuang, Wen
作者单位	1.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Ecol & Environm Sci, 7 Nanhai Rd, Qingdao 266071, Shandong, Peoples R China 2.Univ Calif Riverside, Dept Environm Sci, Riverside, CA 92521 USA 3.Zaozhuang Univ, Coll City & Architecture Engn, Zaozhuang 277160, Shandong, Peoples R China 4.Zaozhuang Univ, Coll Life Sci, Zaozhuang 277160, Shandong, Peoples R China 5.Wuhan Inst Technol, Natl Engn & Technol Res Ctr Dev & Utilizat Phosph, Wuhai 430073, Hubei, Peoples R China
第一作者单位	中国科学院海洋研究所
通讯作者单位	中国科学院海洋研究所
推荐引用方式 GB/T 7714	Zhuang, Wen,Ying, Samantha C.,Frie, Alexander L.,et al. Distribution, pollution status, and source apportionment of trace metals in lake sediments under the influence of the South-to-North Water Transfer Project, China[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2019,671:108-118.
APA	Zhuang, Wen.,Ying, Samantha C..,Frie, Alexander L..,Wang, Qian.,Song, Jinming.,...&Lai, Xiaoying.(2019).Distribution, pollution status, and source apportionment of trace metals in lake sediments under the influence of the South-to-North Water Transfer Project, China.SCIENCE OF THE TOTAL ENVIRONMENT,671,108-118.
MLA	Zhuang, Wen,et al."Distribution, pollution status, and source apportionment of trace metals in lake sediments under the influence of the South-to-North Water Transfer Project, China".SCIENCE OF THE TOTAL ENVIRONMENT 671(2019):108-118.

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